A thermo-responsive supramolecular gel and its luminescence enhancement induced by rare earth Y3

Soft Matter
Xinxian MaJincai Wu

Abstract

A new acylhydrazone-functionalized dual benzimidazole derivative gelator (L) was synthesized. L can self-assemble in DMSO-EG (ethylene glycol) or DMF-water mixtures to form a thermo-responsive supramolecular organogel (L-gel). In order to increase the fluorescence intensity of L-gel (DMSO-EG system), L-gel slowly turned into a clear solution upon addition of one equivalent of RE (rare earth) Y3+. Interestingly, this gelator L and Y3+ can be assembled into an enhanced blue-light-emitting supramolecular metallogel (Y@gel) in DMF-water mixtures.

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Citations

Nov 16, 2018·Chemical Communications : Chem Comm·Xinxian MaMinghua Liu
Jul 3, 2019·Chemical Communications : Chem Comm·Kaitlynn M AyersGaël Ung
Feb 18, 2020·Dalton Transactions : an International Journal of Inorganic Chemistry·Binbin ZhangHong Wang
Jan 25, 2019·Gels·Ty Christoff-TempestaJulia H Ortony
Jan 27, 2019·Advanced Materials·Huiqiong WuJianmin Ma
Aug 25, 2020·Chemistry : a European Journal·Isabel S OliveiraEduardo F Marques
Feb 18, 2021·Langmuir : the ACS Journal of Surfaces and Colloids·Zulal ÖzdemirZdeněk Wimmer
Apr 2, 2021·Journal of Chemical Theory and Computation·Zhen LiKenneth M Merz
Oct 31, 2019·Langmuir : the ACS Journal of Surfaces and Colloids·Qi ZhouHong Wang

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Methods Mentioned

BETA
optical

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