ABO3 and A1-x Cx B1-y Dy (O1-z Ez )3 : review of experimental optimisation of thin film perovskites by high-throughput evaporative physical vapour deposition

Chemical Communications : Chem Comm
Samuel Guerin, Brian E Hayden

Abstract

The development of functional perovskites for future technologies can be achieved though the combinatorial synthetic method of evaporative physical vapour deposition (HT-ePVD) which provides a direct low temperature route to anion stoichiometric materials. When combined with the ability to control and vary precisely the composition of thin film libraries of materials, high-throughput methods of screening and characterisation provides a rapid experimental determination of the structure/function relationship. This review of the use of HT-ePVD shows that controlled cationic substitutions in A and/or B sites can easily be explored, as can the effect of anionic substitution. This is exemplified in using this approach for a wide range of perovskite systems, where the tuning of the functional properties through cation substitution has application in a broad range of technologies.

References

Jan 10, 2006·Journal of Combinatorial Chemistry·Samuel Guerin, Brian E Hayden
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