Ammonia capture and flexible transformation of M-2(INA) (M=Cu, Co, Ni, Cd) series materials

Journal of Hazardous Materials
Yang ChenJiangfeng Yang

Abstract

With the conflicting problems of pollution due to ammonia emissions and the demand for ammonia, we propose M-2(INA) (M=Cu, Co, Ni, Cd) (INA=isonicotinic acid), a series of materials that exhibit flexible conversion in ammonia adsorption. They can capture both wet and dry ammonia for recycling. The materials were obtained by dehydration of coordination materials M(INA)2(H2O)4 (M=Cu, Co, Ni, Cd) (150°C) at atmospheric pressure for 2h. M-2(INA) could reversibly transform to the stable coordination compounds M(INA)2(H2O)2(NH3)2 by adsorbing ammonia in the presence of moisture. The capacity for pure ammonia could reach 12-13mmol/g. Importantly, these materials could stably retain NH3 at a maximum temperature of 80°C and could regenerate below 150°C with no performance loss.

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Citations

Sep 25, 2020·Angewandte Chemie·Dae Won KimChang Seop Hong
May 29, 2021·ACS Applied Materials & Interfaces·Huiyong WangJianji Wang
Feb 10, 2018·Journal of the American Chemical Society·Adam J Rieth, Mircea Dincă
Mar 25, 2020·Chemical Reviews·Timur IslamogluOmar K Farha

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