Baseline characterisation of source contributions to daily-integrated PM2.5 observations at Cape Grim using Radon-222

Environmental Pollution
Jagoda CrawfordArmand J Atanacio

Abstract

We discuss 15 years (2000-2015) of daily-integrated PM2.5 samples from the Cape Grim Station. Ion beam analysis and positive matrix factorisation are used to identify six source-type fingerprints: fresh sea salt (57%); secondary sulfate (14%); smoke (13%); aged sea salt (12%); soil dust (2.4%); and industrial metals (1.5%). An existing hourly radon-only baseline selection technique is modified for use with the daily-integrated observations. Results were not significantly different for days on which >20 hours were below the baseline radon threshold compared with days when all 24 hours satisfied the baseline criteria. This relaxed daily baseline criteria increased the number of samples for analysis by almost a factor of two. Two radon baseline thresholds were tested: historic (100 mBq m-3), and revised (50 mBq m-3). Median aerosol concentrations were similar for both radon thresholds, but maximum values were higher for the 100 mBq m-3 threshold. Back trajectories indicated more interaction with southern Australia and the Antarctic coastline for air masses selected with the 100 mBq m-3 threshold. Radon-only baseline selection using the 50 mBq m-3 threshold was more selective of minimal terrestrial influence than a similar recent s...Continue Reading

References

Nov 26, 2015·Environment International·Chun-Sheng LiangYong-Liang Ma

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Citations

Feb 3, 2021·Journal of Radiological Protection : Official Journal of the Society for Radiological Protection·Yadong Wang

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