Bimetallic metal-organic frameworks and their derivatives.

Chemical Science
Liyu ChenQiang Xu

Abstract

Bimetallic metal-organic frameworks (MOFs) have two different metal ions in the inorganic nodes. According to the metal distribution, the architecture of bimetallic MOFs can be classified into two main categories namely solid solution and core-shell structures. Various strategies have been developed to prepare bimetallic MOFs with controlled compositions and structures. Bimetallic MOFs show a synergistic effect and enhanced properties compared to their monometallic counterparts and have found many applications in the fields of gas adsorption, catalysis, energy storage and conversion, and luminescence sensing. Moreover, bimetallic MOFs can serve as excellent precursors/templates for the synthesis of functional nanomaterials with controlled sizes, compositions, and structures. Bimetallic MOF derivatives show exposed active sites, good stability and conductivity, enabling them to extend their applications to the catalysis of more challenging reactions and electrochemical energy storage and conversion. This review provides an overview of the significant advances in the development of bimetallic MOFs and their derivatives with special emphases on their preparation and applications.

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Citations

Feb 19, 2021·Accounts of Chemical Research·Hanna L B Boström, Andrew L Goodwin
Oct 13, 2020·Organic & Biomolecular Chemistry·Yu WangQiang Xu
Jan 7, 2021·ACS Applied Materials & Interfaces·Tomislav StolarKrunoslav Užarević
May 30, 2021·Advanced Materials·Yu ShenFengwei Huo

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Methods Mentioned

BETA
X-ray
thermal treatment

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