Comparison of holographic photopolymer materials by use of analytic nonlocal diffusion models

Applied Optics
Feidhlim T O'NeillJohn T Sheridan

Abstract

The one-dimensional diffusion equation governing holographic grating formation in photopolymers, which includes both nonlocal material response and generalized dependence of the rate of polymerization on the illuminating intensity, has been previously solved under the two-harmonic expansion assumption. The resulting analytic expressions for the monomer and polymer concentrations have been derived and their ranges of validity tested in comparison with the more accurate numerical four-harmonic case. We used these analytic expressions to carry out a study of experimental results presented in the literature over a 30-year period. Automatic fitting of the data with these formulas allows material parameters, including the nonlocal chain-length variance sigma, to be estimated. In this way, (i) a quantitative comparison of different materials can be made, and (ii) a standard form of experimental result presentation is proposed to facilitate such a procedure.

References

Jun 13, 2000·Journal of the Optical Society of America. A, Optics, Image Science, and Vision·J T Sheridan, J R Lawrence
Jul 1, 1971·Applied Optics·W S Colburn, K A Haines
Mar 1, 1975·Applied Optics·B L Booth
Sep 15, 1987·Applied Optics·S Calixto
Jul 10, 1993·Applied Optics·A FimiaF Amat-Guerri

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