PMID: 11909055Mar 23, 2002Paper

Constant bond breakup probability model for reversible aggregation processes

Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics
Gerardo OdriozolaR Hidalgo-Alvarez

Abstract

Reversible aggregation processes were simulated for systems of freely diffusing sticky particles. Reversibility was introduced by allowing that all bonds in the system may break with a given probability per time interval. In order to describe the kinetics of such aggregation-fragmentation processes, a fragmentation kernel was developed and then used together with the Brownian aggregation kernel for solving the corresponding kinetic master equation. The deduced fragmentation kernel considers a single characteristic lifetime for all bonds and accounts for the cluster morphology by averaging over all possible configurations for clusters of a given size. It became evident that the simulated cluster-size distributions could be described only when an additional fragmentation effectiveness was considered. Doing so, the stochastic solutions were in good agreement with the simulated data.

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Citations

Oct 14, 2011·The Journal of Chemical Physics·Gerardo Odriozola
Aug 11, 2007·The Journal of Chemical Physics·Sujin BabuTaco Nicolai
May 23, 2012·Journal of Controlled Release : Official Journal of the Controlled Release Society·Chinmay PangarkarSamir Mitragotri
Dec 17, 2008·Advances in Colloid and Interface Science·Nina KovalchukNidal Hilal
May 9, 2006·Magnetic Resonance Imaging·Mikhail G ShapiroAlan Jasanoff
Jun 24, 2016·The Journal of Chemical Physics·Nitin S Tiwari, Paul van der Schoot
Sep 9, 2004·The Journal of Chemical Physics·G OdriozolaR Hidalgo-Alvarez
Mar 1, 2006·The European Physical Journal. E, Soft Matter·S BabuD Durand
Jul 23, 2019·Physical Chemistry Chemical Physics : PCCP·A Arango-RestrepoJ M Rubi
Jan 17, 2020·Scientific Reports·Erzsébet Bartolák-Suki, Béla Suki
May 5, 2012·Chemphyschem : a European Journal of Chemical Physics and Physical Chemistry·Teresa López-LeónDelfina Bastos-González
Jul 18, 2020·Nature Communications·Joep RouwhorstPeter Schall
Jul 7, 2011·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Qiang Chang, Jin Yang
May 16, 2007·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·J C Fernández-ToledanoR Hidalgo-Alvarez
May 3, 2021·Advances in Colloid and Interface Science·Ivanna Colijn, Karin Schroën
Mar 24, 2007·Journal of Colloid and Interface Science·G OdriozolaR Hidalgo-Alvarez
Apr 28, 2007·The Journal of Physical Chemistry. B·Antonio M Puertas, Gerardo Odriozola

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