PMID: 15244797Jul 13, 2004Paper

Cooling rate, heating rate, and aging effects in glassy water

Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics
Nicolas GiovambattistaFrancesco Sciortino

Abstract

We report a molecular dynamics simulation study of the properties of the potential energy landscape sampled by a system of water molecules during the process of generating a glass by cooling, and during the process of regenerating the equilibrium liquid by heating the glass. We study the dependence of these processes on the cooling/heating rates as well as on the role of aging (the time elapsed in the glass state). We compare the properties of the potential energy landscape sampled during these processes with the corresponding properties sampled in the liquid equilibrium state to elucidate under which conditions glass configurations can be associated with equilibrium liquid configurations.

References

Oct 4, 2000·Physical Review Letters·S Buchner, A Heuer
Mar 22, 2001·Nature·P G Debenedetti, F H Stillinger
Aug 11, 2001·Physical Review Letters·L AngelaniG Ruocco
Nov 13, 2003·Physical Review Letters·Francesco SciortinoPiero Tartaglia
Mar 31, 1995·Science·C A Angell

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Citations

Feb 21, 2006·Physical Review Letters·Brittany A Isner, Daniel J Lacks
Jun 17, 2019·The Journal of Chemical Physics·Nicolas GiovambattistaPeter H Poole
Aug 25, 2004·Physical Review Letters·Nicolas GiovambattistaH Eugene Stanley
Aug 11, 2005·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Nicolas GiovambattistaH Eugene Stanley
Oct 26, 2005·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Nicolas GiovambattistaFrancesco Sciortino
Feb 9, 2005·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Vo Van Hoang, Suhk Kun Oh
May 21, 2005·Physical Review Letters·M M KozaT Hansen
Aug 11, 2005·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Nicolas GiovambattistaH Eugene Stanley
Aug 16, 2006·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Hans Christian Ottinger
Apr 2, 2021·Proceedings of the National Academy of Sciences of the United States of America·Loni KringleGreg A Kimmel
Jun 9, 2021·Nature Communications·Thomas E GartnerPablo G Debenedetti

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