PMID: 25790221DOI: 10.1039/c5cc01560jMar 20, 2015Paper
"Decarbonization" of an imino-N-heterocyclic carbene ligand via triple benzyl migration from hafnium
Chemical Communications : Chem Comm
Dipesh PremaLeGrande M Slaughter
Abstract
An imino-N-heterocyclic carbene underwent three sequential benzyl migrations upon reaction with tetrabenzylhafnium, resulting in complete removal of the carbene carbon from the ligand. The resulting eneamido-amidinato hafnium complex showed alkene polymerization activity comparable to that of a precatalyst containing the intact iminocarbene ligand.
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