Donor-acceptor-type supramolecular polymers on the basis of preorganized molecular tweezers/guest complexation

Chemical Society Reviews
Yifei HanFeng Wang

Abstract

The bottom-up self-assembly of donor-acceptor (D-A) units has received tremendous attention in recent years. Charge-transfer interactions, which are inherently embedded in D-A pairs, have suffered from some disadvantages such as erratic arrangements and weak binding affinity, thus hampering the precise arrangement of D-A units into long-range-ordered supramolecular polymers. To address this issue, a feasible protocol is to incorporate D-A units into molecular tweezers/guest recognition motifs, which concurrently feature high complexation directionality, strong binding affinity and stimuli-responsiveness. In this tutorial review, we have summarized the recent advances on the tweezering directed formation of D-A-type supramolecular polymers, with particular emphasis on the design principles of monomers and macroscopic behaviors of supramolecular polymers, together with future challenges in this research field.

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Citations

Aug 17, 2018·Chemical Communications : Chem Comm·Zongchun GaoFeng Wang
Nov 13, 2018·Chemical Communications : Chem Comm·Hui LiWei Tian
May 12, 2019·Molecules : a Journal of Synthetic Chemistry and Natural Product Chemistry·Amira MbarekJeanne Leblond Chain
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Jan 16, 2021·Angewandte Chemie·Zijian LiFeng Wang
Feb 11, 2020·Journal of the American Chemical Society·Huiqing LiYun-Bao Jiang
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Jan 8, 2022·Chemical Communications : Chem Comm·Hye Jin JangKyu-Sung Jeong

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Methods Mentioned

BETA
1
H
NMR
scanning electron microscopy
X-ray
AFM

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