Effect of Ag nanoparticle concentration on the electrical and ferroelectric properties of Ag/P(VDF-TrFE) composite films

Scientific Reports
Haemin PaikKwangsoo No

Abstract

We investigated the effect of the Ag nanoparticles on the ferroelectric and piezoelectric properties of Ag/poly(vinylidenefluoride-trifluoroethylene) (P(VDF-TrFE)) composite films. We found that the remanent polarization and direct piezoelectric coefficient increased up to 12.14 μC/cm(2) and 20.23 pC/N when the Ag concentration increased up to 0.005 volume percent (v%) and decreased down to 9.38 μC/cm(2) and 13.45 pC/N when it increased up to 0.01 v%. Further increase in Ag concentration resulted in precipitation of Ag phase and significant leakage current that hindered any meaningful measurement of the ferroelectric and piezoelectric properties. 46% increase of the remanent polarization value and 27% increase of the direct piezoelectric coefficient were observed in the film with the 0.005 v% of the Ag nanoparticles added without significant changes to the crystalline structure confirmed by both X-ray diffraction (XRD) and Fourier transform infrared (FT-IR) experiments. These enhancements of both the ferroelectric and piezoelectric properties are attributed to the increase in the effective electric field induced by the reduction in the effective volume of P(VDF-TrFE) that results in more aligned dipoles.

Citations

Aug 11, 2017·Nihon yakurigaku zasshi. Folia pharmacologica Japonica·Yuhei Nishimura
Jul 14, 2021·Advanced Science·Susmriti Das MahapatraVijay Kumar Thakur
Dec 27, 2017·ACS Applied Materials & Interfaces·Deepa SinghAshish Garg
Apr 10, 2019·ACS Applied Materials & Interfaces·Soaram KimGoutam Koley
Aug 19, 2020·Analytical Chemistry·Agnieszka PriebeJohann Michler

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BETA
scanning electron microscopy
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