Efficient removal of arsenite by a composite of amino modified silica supported MnO2/Fe-Al hydroxide (SNMFA) prepared from biotite.

Journal of Environmental Management
Qiang ZengLiang Hu

Abstract

Developing materials from natural minerals to efficiently remove arsenite (As(Ⅲ)) from solution is vital important for resources comprehensive utilization and environment protection. In this study, biotite containing minerals was used to prepare a novel composite of amino modified silica supported MnO2/Fe-Al hydroxide (SNMFA composite), which was then applied to remove arsenite. Scanning electron microscope (SEM), X-ray diffraction (XRD) and X-ray photoelectron spectroscopy (XPS) results indicated that many amorphous MnO2 and Fe-Al hydroxide nano sheets were loaded on the surface of layered silica structure. Batch experiments showed that this composite could efficiently remove As(Ⅲ) from aqueous solution, and the maximal removal capacity was identified as 46.11 mg/g. As(Ⅲ) adsorption behaviours of SNMFA composite were confirmed by the pseudo-second-order kinetic model and Langmuir model, indicating that As(Ⅲ) adsorption on its surface was monolayer adsorption. The adsorption process was a pH and temperature dependent process, and increasing pH and temperature have facilitated the removal of As(Ⅲ). Thermodynamic analysis showed that As(Ⅲ) adsorption process was a spontaneous endothermic reaction. The As(Ⅲ) removal was mainly rel...Continue Reading

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