Electrodeposition of ZnO window layer for an all-atmospheric fabrication process of chalcogenide solar cell

Scientific Reports
Fabien TsinJean Rousset

Abstract

This paper presents the low cost electrodeposition of a transparent and conductive chlorine doped ZnO layer with performances comparable to that produced by standard vacuum processes. First, an in-depth study of the defect physics by ab-initio calculation shows that chlorine is one of the best candidates to dope the ZnO. This result is experimentally confirmed by a complete optical analysis of the ZnO layer deposited in a chloride rich solution. We demonstrate that high doping levels (>10(20) cm(-3)) and mobilities (up to 20 cm(2) V(-1) s(-1)) can be reached by insertion of chlorine in the lattice. The process developed in this study has been applied on a CdS/Cu(In,Ga)(Se,S)2 p-n junction produced in a pilot line by a non vacuum process, to be tested as solar cell front contact deposition method. As a result efficiency of 14.3% has been reached opening the way of atmospheric production of Cu(In,Ga)(Se,S)2 solar cell.

References

Oct 24, 2013·Advanced Materials·Harald HagendorferAyodhya N Tiwari

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Citations

Jun 15, 2016·ACS Applied Materials & Interfaces·Mingqing Wang, Kwang-Leong Choy
Oct 25, 2016·Journal of Materials Chemistry. A, Materials for Energy and Sustainability·Xin RenJudith L MacManus-Driscoll
Aug 30, 2017·Physical Chemistry Chemical Physics : PCCP·Jorge L Cholula-DíazPablo Esquinazi
Mar 11, 2021·ACS Applied Materials & Interfaces·Van Ben ChuPhillip J Dale
Apr 27, 2019·ACS Applied Materials & Interfaces·Joel van Embden, Enrico Della Gaspera

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Methods Mentioned

BETA
thermal treatment
X-ray

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NEXCIS

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