Emission characteristics of PCDD/Fs in stack gas from municipal solid waste incineration plants in Northern China

Chemosphere
Feng ZhuChengyang Hong

Abstract

Emission characteristics including congener's profile, gas emissions and toxic equivalent concentration (TEQ) indicators of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) in 57 stack gas samples from 6 municipal solid waste incinerators (MSWIs) in Northern China were investigated by gas chromatography-high resolution mass spectrometry (HRGC-HRMS). Additionally, PCDD/Fs formation mechanisms from the MSWIs were briefly discussed. Results revealed that the concentrations and equivalent concentrations of PCDD/Fs emissions in stack gas from 6 MSWIs were in the range of 0.11-2.53 ng Nm-3and 0.007-0.059 ng TEQ Nm-3, respectively. The emission factors of PCDD/Fs from 6 MSWIs varied from 0.027 to 0.225 μg I-TEQ tonne-1, with a mean value of 0.17 μg I-TEQ tonne-1waste, which was estimated to an annual emission of 234.96 mg I-TEQ of PCDD/Fs from 6 MSWIs to the atmosphere. O8CDD, O8CDF and 1,2,3,4,6,7,8-H7CDD were the indicatory compounds of PCDD/Fs to apportion the sources of PCDD/Fs in environmental medium especially in ambient environment of MSWIs. 1,2,3,7,8,9-H6CDF and 1,2,3,4,7,8-H6CDF can be used as TEQ indicators for monitoring PCDD/Fs emission. Based on the positive matrix factorization (PMF) model, eight factors wer...Continue Reading

Citations

Jun 20, 2020·Environmental Science and Pollution Research International·Tong Chen Qiang-Yu
Feb 8, 2019·Environmental Science and Pollution Research International·Mingxiu ZhanXiaodong Li
Apr 12, 2019·International Journal of Environmental Research and Public Health·Gang ZhangJing Hai

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