Engineering the Interfaces of Superadsorbing Graphene-Based Electrodes with Gas and Electrolyte to Boost Gas Evolution and Activation Reactions

ChemSusChem
Jun-Jun ZhangJie-Sheng Chen

Abstract

Electrochemical gas evolution and activation reactions are complicated processes, involving not only active electrocatalysts but also the interaction among solid electrodes, electrolyte, and gas-phase products and reactants. In this study, multiphase interfaces of superadsorbing graphene-based electrodes were controlled without changing the active centers to significantly facilitate mass diffusion kinetics for superior performance. The achieved in-depth understanding of how to regulate the interfacial properties to promote the electrochemical performance could provide valuable clues for electrode manufacture and for the design of more active electrocatalysts.

References

May 25, 2011·Advanced Materials·Myung-Hyun RyouJang Wook Choi
Aug 22, 2012·Angewandte Chemie·Xin-Hao LiMarkus Antonietti
May 24, 2014·Angewandte Chemie·Tian-Nan YeJie-Sheng Chen
Jun 5, 2014·Chemical Reviews·Adriano AmbrosiMartin Pumera
Mar 3, 2015·Advanced Materials·Zhiyi LuLei Jiang
May 6, 2017·Chemistry : a European Journal·Mao MiaoXin Wang
Aug 31, 2017·Journal of the American Chemical Society·Xia ShengLei Jiang

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Citations

Mar 16, 2019·Chemical Communications : Chem Comm·Jun-Jun ZhangJie-Sheng Chen
Nov 12, 2020·Chemical Communications : Chem Comm·Jun-Jun ZhangNan-Nan Zhang
Mar 12, 2021·Chemical Communications : Chem Comm·Jun-Jun ZhangNan-Nan Zhang

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