Evaluation of biochars in reducing the bioavailability of flubendiamide in water/sediment using passive sampling with polyoxymethylene

Journal of Hazardous Materials
Pingping WangYongquan Zheng

Abstract

An equilibrium passive sampler based on POM was first used to determine the Cfree of flubendiamide in water/sediment systems. The adsorption of flubendiamide by POM followed a first-order one-compartment uptake model and the POM-water partition coefficient was 1.90. The method was used to compare the efficiency of three biochars which were produced from crofton weed (BC-1, ∼500°C), macadamia (BC-2, 550-660°C) and wheat straw (BC-3, 550°C). The Freundlich fit the sorption isotherm data well and the adsorption capacity was BC-1>BC-3>BC-2. The percent removal of the BC-1 was higher in acidic solutions. When different doses of BC-1 were added to two sediments, the Cfree of the flubendiamide was higher in the sediment with a low organic matter content (S-1). With an increase of BC-1, the Cfree was significantly reduced in S-1. A 30-day period of biochar-sediment contact time was sufficient for a reduction of freely dissolved flubendiamide in the case of the two sediments tested. In the combination of biochar addition (5%) and aging time (30days), the maximum reductions were 87% and 60% in S-1 and S-2. Therefore, the reduction of bioavailability of the flubendiamide and pollution repair can be achieved by this process.

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