Exact Potential Driving the Electron Dynamics in Enhanced Ionization of H_{2}^{+}

Physical Review Letters
Elham KhosraviNeepa T Maitra

Abstract

It was recently shown that the exact factorization of the electron-nuclear wave function allows the construction of a Schrödinger equation for the electronic system, in which the potential contains exactly the effect of coupling to the nuclear degrees of freedom and any external fields. Here we study the exact potential acting on the electron in charge-resonance enhanced ionization in a model one-dimensional H_{2}^{+} molecule. We show there can be significant differences between the exact potential and that used in the traditional quasistatic analyses, arising from nonadiabatic coupling to the nuclear system, and that these are crucial to include for accurate simulations of time-resolved ionization dynamics and predictions of the ionization yield.

References

Oct 1, 1988·Physical Review A: General Physics·J JavanainenQ Su
Nov 1, 1993·Physical Review. a·T ZuoA D Bandrauk
Apr 1, 1996·Physical Review. a·K C KulanderK J Schafer
Oct 9, 1995·Physical Review Letters·T SeidemanP B Corkum
May 27, 1996·Physical Review Letters·E ConstantP B Corkum
Apr 6, 2001·Physical Review Letters·T Kreibich, E K Gross
Oct 4, 2003·Physical Review Letters·F LégaréP B Corkum
Apr 2, 2008·The Journal of Chemical Physics·L S Cederbaum
Oct 10, 2008·The Journal of Physical Chemistry. B·Sharon Hammes-Schiffer, Alexander V Soudackov
Sep 28, 2010·Physical Review Letters·Ali AbediE K U Gross
Jan 15, 2011·Physical Review Letters·Norio Takemoto, Andreas Becker
Sep 10, 2011·Physical Review Letters·Irina BocharovaFrançois Légaré
Dec 20, 2012·The Journal of Chemical Physics·Ali AbediE K U Gross
Jun 21, 2013·The Journal of Chemical Physics·Lorenz S Cederbaum
Feb 12, 2014·Philosophical Transactions. Series A, Mathematical, Physical, and Engineering Sciences·Nikitas I Gidopoulos, E K U Gross
Jan 24, 2015·Physical Review Letters·Seung Kyu MinE K U Gross
Mar 3, 2015·The Journal of Chemical Physics·Federica AgostiniE K U Gross
Aug 12, 2015·The Journal of Physical Chemistry Letters·G J HalászL S Cederbaum

❮ Previous
Next ❯

Citations

Apr 1, 2016·Journal of Chemical Theory and Computation·Federica AgostiniEberhard K U Gross
Jul 28, 2016·The Journal of Chemical Physics·Basile F E CurchodE K U Gross
Feb 6, 2017·The Journal of Physical Chemistry Letters·Basile F E Curchod, Federica Agostini
Jun 18, 2017·The Journal of Physical Chemistry Letters·Seung Kyu MinE K U Gross
Aug 10, 2017·Physical Chemistry Chemical Physics : PCCP·Ryoji AnzakiKenichi L Ishikawa
Mar 3, 2017·The Journal of Chemical Physics·Mu-Zi LiXue-Bin Bian
Apr 22, 2019·The Journal of Chemical Physics·Graeme H GosselNeepa T Maitra
May 6, 2017·Physical Review Letters·Axel Schild, E K U Gross
Feb 8, 2020·Physical Review Letters·Francesco TalottaFederica Agostini
Jan 9, 2021·The Journal of Chemical Physics·Phillip MartinezNeepa T Maitra
Mar 24, 2021·The Journal of Chemical Physics·Marco SchiròFederica Agostini
Dec 10, 2016·The Journal of Physical Chemistry. a·A TóthÁ Vibók
Aug 1, 2018·Journal of Chemical Theory and Computation·Graeme H GosselNeepa T Maitra
Aug 14, 2020·The Journal of Physical Chemistry. a·Francesco TalottaGiovanni Ciccotti

❮ Previous
Next ❯

Related Concepts

Trending Feeds

COVID-19

Coronaviruses encompass a large family of viruses that cause the common cold as well as more serious diseases, such as the ongoing outbreak of coronavirus disease 2019 (COVID-19; formally known as 2019-nCoV). Coronaviruses can spread from animals to humans; symptoms include fever, cough, shortness of breath, and breathing difficulties; in more severe cases, infection can lead to death. This feed covers recent research on COVID-19.

Blastomycosis

Blastomycosis fungal infections spread through inhaling Blastomyces dermatitidis spores. Discover the latest research on blastomycosis fungal infections here.

Nuclear Pore Complex in ALS/FTD

Alterations in nucleocytoplasmic transport, controlled by the nuclear pore complex, may be involved in the pathomechanism underlying multiple neurodegenerative diseases including Amyotrophic Lateral Sclerosis and Frontotemporal Dementia. Here is the latest research on the nuclear pore complex in ALS and FTD.

Applications of Molecular Barcoding

The concept of molecular barcoding is that each original DNA or RNA molecule is attached to a unique sequence barcode. Sequence reads having different barcodes represent different original molecules, while sequence reads having the same barcode are results of PCR duplication from one original molecule. Discover the latest research on molecular barcoding here.

Chronic Fatigue Syndrome

Chronic fatigue syndrome is a disease characterized by unexplained disabling fatigue; the pathology of which is incompletely understood. Discover the latest research on chronic fatigue syndrome here.

Evolution of Pluripotency

Pluripotency refers to the ability of a cell to develop into three primary germ cell layers of the embryo. This feed focuses on the mechanisms that underlie the evolution of pluripotency. Here is the latest research.

Position Effect Variegation

Position Effect Variagation occurs when a gene is inactivated due to its positioning near heterochromatic regions within a chromosome. Discover the latest research on Position Effect Variagation here.

STING Receptor Agonists

Stimulator of IFN genes (STING) are a group of transmembrane proteins that are involved in the induction of type I interferon that is important in the innate immune response. The stimulation of STING has been an active area of research in the treatment of cancer and infectious diseases. Here is the latest research on STING receptor agonists.

Microbicide

Microbicides are products that can be applied to vaginal or rectal mucosal surfaces with the goal of preventing, or at least significantly reducing, the transmission of sexually transmitted infections. Here is the latest research on microbicides.