Fine particle attachment to quartz sand in the presence of multiple interacting dissolved components

The Science of the Total Environment
Zahra Sadat RastghalamBradley Freake

Abstract

In natural aquatic systems water chemistry is complicated and fine particles encounter multiple water components simultaneously, yet the combined effects of some multiple components on the fate and transport of these particles have not been elucidated. In this study nTiO2 and illite colloid attachment to quartz sand was investigated in 1 mM NaCl and 0.5 mM CaCl2 background solutions using a range of phosphate concentrations (0 to 10 mg/L) at pH 5 and 9. The results obtained from the batch experiments indicated that without using phosphate, nTiO2 aggregation and attachment was strongly influenced by pH and Ca2+, both of which modified nTiO2 surface charges. nTiO2 attachment was high in CaCl2 solution at pH 9 due to attractive forces between nTiO2 and sand, as well as ripening. Furthermore, phosphate adsorption to nTiO2 was higher in CaCl2 solution at pH 9 than that at pH 5 due to attractive forces between nTiO2 and phosphate anions, and also potential surface precipitation of Ca-P minerals at pH 9. Phosphate adsorption to illite was low owing to strong repulsive forces between illite and phosphate. The effect of phosphate on nTiO2 and illite attachment to sand was influenced by pH and cation valency. A decreasing trend in nTiO2 ...Continue Reading

Citations

Sep 8, 2020·Environmental Monitoring and Assessment·A BaysalG S Ustabasi
Apr 19, 2021·The Science of the Total Environment·Marie SimoninAgnès Richaume

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