From Isolated Ions to Multilayer Functional Materials Using Ion Soft Landing

Angewandte Chemie
Julia LaskinVenkateshkumar Prabhakaran

Abstract

The ability to deposit intact polyatomic ions with well-defined composition, charge state, and kinetic energy onto surfaces makes preparative mass spectrometry, also called ion soft landing, particularly attractive for preparing uniform molecular and ionic layers. Early studies characterized the structures, charge states, and reactivity of sparsely distributed soft-landed species. The recent development of high-flux ionization sources has opened up new opportunities for the precisely controlled preparation of both two-dimensional structures and three-dimensional multilayer architectures by ion soft landing. The deposition of large numbers of ions onto supports led to previously unknown phenomena being uncovered, thereby opening several exciting research directions. Furthermore, faster ion deposition has enabled fabrication of novel functional devices. This Review discusses important phenomena and highlights key developments pertaining to the preparation of well-defined interfaces for studies in energy storage, catalysis, soft materials, and biology.

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May 10, 2019·Physical Chemistry Chemical Physics : PCCP·Matthew R HenryAndrei G Fedorov
Dec 18, 2019·Physical Chemistry Chemical Physics : PCCP·Ethan P KamphausPerla B Balbuena
Jul 2, 2019·Angewandte Chemie·Archismita MisraMay Nyman
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Sep 4, 2020·Proceedings of the National Academy of Sciences of the United States of America·Jonas WarnekeJulia Laskin
Feb 29, 2020·Angewandte Chemie·Pei SuJulia Laskin
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May 21, 2021·Chemistry : a European Journal·Martin MayerJonas Warneke
Aug 19, 2020·Journal of the American Society for Mass Spectrometry·Pei SuJulia Laskin
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Apr 20, 2019·Analytical Chemistry·Pei SuJulia Laskin
Sep 23, 2021·The Journal of Physical Chemistry Letters·Kie HankinsVijayakumar Murugesan
Sep 16, 2021·Angewandte Chemie·Fangshun YangJonas Warneke
Oct 22, 2021·Analytical Chemistry·Hugo Y Samayoa-OviedoJulia Laskin

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