Functional π-Conjugated Two-Dimensional Covalent Organic Frameworks

ACS Applied Materials & Interfaces
H Vignesh BabuM Rajeswara Rao

Abstract

Fingerprints of π-conjugated compounds are ubiquitous in nature and play a crucial part in human existence. For instance, cis-retinal, an endogenous π-conjugated molecule present in the eye, performs a vital role in the function of visual perception. π-Conjugated molecules have also received a great deal of attention owing to their intriguing optical properties and created a surge in optoelectronics. Varieties of π-conjugated molecules/oligomers have been developed and explored for a number of applications such as organic light-emitting diodes (OLEDs), organic field-effect transistors (OFETs), organic photovoltaics (OPVs), and sensors, among others. While the extended π-delocalization in one-dimensional (1D) polymers versus oligomers produce superior optical and electronic properties, further extension of π-delocalization to the second dimension (2D) is expected to give rise even more intriguing properties as revealed by theoretical studies. As a matter of fact, graphene is the best example of 2D-conjugated polymers, but its zero-band-gap behavior is a major impediment for semiconducting applications. In contrast, it was challenging to prepare 2D crystalline polymers until the discovery of boroxine/boronate ester linked covalen...Continue Reading

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Feb 19, 2020·Chemical Society Reviews·Xinyu GuanShilun Qiu
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