Functional Supramolecular Architectures of Dipyrrin Complexes

Frontiers in Chemistry
Ryota Matsuoka, Tatsuya Nabeshima

Abstract

Dynamic formation of self-assemblies from molecular components is a useful and efficient way to produce molecular and supramolecular architectures with sophisticated functions. The labile coordination bond and dynamic covalent bond as a reversible bond have often been used to create a well-organized supramolecular self-assembly. In order to realize sophisticated novel functions of the supramolecular self-assemblies, dipyrrin complexes have recently been employed as a functional unit and incorporated into the supramolecular architectures because of their outstanding properties and functions such as a high photostability and strong light absorption/emission. This review article summarizes recent development in functional supramolecular architectures of the dipyrrin complexes produced by coordination to a metal ion and dynamic covalent bond formation. We first describe the synthesis and unique functions of a series of discrete supramolecular architectures: helicates, macrocycles, and cages. The polymeric supramolecular self-assemblies with 1D, 2D, and 3D structures are then introduced as a functional infinite supramolecular architecture.

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Citations

Mar 1, 2019·Dalton Transactions : an International Journal of Inorganic Chemistry·Fan ZhangMir Wais Hosseini
Feb 14, 2020·Physical Chemistry Chemical Physics : PCCP·Barry ManghamNeil R Champness
Apr 21, 2020·Dalton Transactions : an International Journal of Inorganic Chemistry·Stéphane A Baudron
Feb 23, 2021·Chemical Record : an Official Publication of the Chemical Society of Japan ... [et Al.]·Isha MishraMalaichamy Sathiyendiran
Dec 7, 2021·Accounts of Chemical Research·Elisa Tomat, Clayton J Curtis

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Methods Mentioned

BETA
X-ray
NMR

Software Mentioned

BODIPY

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