PMID: 11909355Mar 23, 2002Paper

Generation of single dispersion precompensated 1-fs pulses by shaped-pulse optimized high-order stimulated Raman scattering

Physical Review Letters
V P KaloshaMisha Ivanov

Abstract

We propose and theoretically analyze a new approach for generating and shaping 1-fs pulses. It combines the ideas of strong-field molecular optics and optimal control to manipulate light generation in a pump-probe Raman regime. Flexible phase control over the generated spectrum of about 3 eV width is achieved by controlling the input pulses and maximizing the coherence of medium excitation by adiabatically aligning molecules in the medium with a specially shaped pump pulse. The generated pulse is optimized for an output window, precompensating for its dispersion to all orders.

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Citations

Feb 11, 2012·The Journal of Chemical Physics·Zhiying Li, Eric J Heller
Jul 13, 2005·The Journal of Chemical Physics·Yoshi-Ichi Suzuki, Tamar Seideman
Sep 8, 2011·The Journal of Chemical Physics·E Gershnabel, I Sh Averbukh
Sep 15, 2014·The Journal of Chemical Physics·Zhiying LiEric J Heller
Jul 21, 2004·The Journal of Chemical Physics·Mikael D PoulsenTamar Seideman
Jul 23, 2004·The Journal of Chemical Physics·Giovanni GranucciPiet Van Leuven
May 16, 2003·Optics Letters·Michael SpannerMaxim Pshenichnikov
Apr 20, 2004·Physical Review Letters·Michael SpannerMisha Ivanov
Jun 21, 2011·Optics Letters·V A PolovinkinOlga Kocharovskaya
May 31, 2014·Optics Letters·Gennady RasskazovMarcos Dantus
Nov 21, 2007·Optics Letters·Sergey YeremenkoDouwe A Wiersma
Jun 6, 2003·Physical Review Letters·M LeibscherH Rabitz
Apr 8, 2021·Spectrochimica Acta. Part A, Molecular and Biomolecular Spectroscopy·Vijit V NautiyalVinod Prasad
Sep 28, 2017·The Journal of Physical Chemistry Letters·Dina RosenbergSharly Fleischer

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