Heterodyne spectral interferometry for multidimensional nonlinear spectroscopy of individual quantum systems

Optics Letters
W Langbein, Brian Patton

Abstract

A novel implementation of transient nonlinear spectroscopy is presented that allows the study of the transient nonlinear polarization emitted from individual electronic transitions. Both the amplitude and the phase of the polarization are retrieved, permitting the implementation of multidimensional spectroscopy in the excitation pulse delays. The technique is shown to detect mutual coherent coupling in a group of individual, localized excitonic transitions.

References

Jun 7, 2003·Science·Peifang TianWarren S Warren
May 4, 2004·Optics Letters·T BrixnerG R Fleming
Apr 1, 2005·Nature·Tobias BrixnerGraham R Fleming
Aug 11, 2005·Physical Review Letters·Wolfgang Langbein, Brian Patton
Jan 12, 2008·Optics Letters·M F EmdeD A Wiersma

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Citations

Mar 8, 2013·The Review of Scientific Instruments·P DeyD Karaiskaj
Aug 7, 2009·The Review of Scientific Instruments·A D BristowS T Cundiff
Apr 25, 2013·Nature Communications·F AlbertW Langbein
Jul 25, 2007·Journal of Physics. Condensed Matter : an Institute of Physics Journal·Paola Borri, Wolfgang Langbein
Jul 25, 2007·Journal of Physics. Condensed Matter : an Institute of Physics Journal·Wolfgang Langbein, Brian Patton
Mar 9, 2010·Nature Materials·J KasprzakW Langbein
Feb 15, 2020·Optics Letters·Daniel WiggerJacek Kasprzak
Apr 7, 2021·Optics Express·Yasuyoshi MitsumoriKeiichi Edamatsu
Jun 12, 2021·Physical Review Letters·Christopher L SmallwoodSteven T Cundiff
Oct 31, 2021·Advanced Science·Thilo HahnDaniel Wigger

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