High-performance nanofiltration membranes with a sandwiched layer and a surface layer for desalination and environmental pollutant removal

The Science of the Total Environment
Langming BaiHeng Liang

Abstract

To overcome the permeability-selectivity limitation and improve the performance of desalination membranes, novel methods and design strategies are needed to prepare new types of thin film composite (TFC) nanofiltration (NF) membranes. In this work, a modified TFC membrane with a sandwiched layer and a surface layer was fabricated through a facile additional two-step approach. The microfiltration (MF) substrate and TFC surface were modified by a cellulose nanocrystal (CNC) sandwiched layer and a polydopamine (PDA) layer, respectively. Scanning electron microscopy (SEM) analysis indicated that the support modified by CNCs presented a more homogeneous surface than the control TFC. Cross-sectional SEM images showed that the underneath MF support, CNC interlayer, polyamide layer and PDA deposition layer were perfectly integrated. The surface charge was determined by an electrophoretic analyzer and revealed that the CNC interlayer increased the membrane electronegativity, while the PDA layer presented the opposite effect. Compared to the control TFC membrane, the solute permeability and rejection of the resultant CNC-TFC-PDA membrane were simultaneously increased, indicating a breakthrough in the trade-off limitation. The modified me...Continue Reading

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