Highly crystalline MOF-based materials grown on electrospun nanofibers

Nanoscale
M BechelanyP Miele

Abstract

Supported Metal Organic Frameworks (MOFs) with a high specific surface area are of great interest for applications in gas storage, separation, sensing, and catalysis. In the present work we report the synthesis of a novel composite architecture of MOF materials supported on a flexible mat of electrospun nanofibers. The system, based on three-dimensional interwoven nanofibers, was designed by using a low-cost and scalable multistep synthesis protocol involving a combination of electrospinning and low-temperature atomic layer deposition of oxide materials, and their subsequent solvothermal conversion under either conventional or microwave-assisted heating. This highly versatile approach allows the production of different types of supported MOF crystals with controlled sizes, morphology, orientation and high accessibility.

References

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Jan 27, 2012·Advanced Materials·Catherine MarichyNicola Pinna
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Nov 10, 2013·Beilstein Journal of Nanotechnology·Adib Abou ChaayaPhilippe Miele
Jun 27, 2014·Chemical Society Reviews·Shilun QiuGuangshan Zhu

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Citations

Mar 24, 2016·ACS Applied Materials & Interfaces·Martin DrobekSang Sub Kim
Dec 11, 2019·Nanomaterials·Ana Cláudia Canalli BortolassiMikhael Bechelany
Mar 1, 2019·Nanomaterials·Paulina ListewnikMałgorzata Jędrzejewska-Szczerska
Feb 14, 2016·Journal of Materials Chemistry. B, Materials for Biology and Medicine·Sakthivel NagarajanSébastien Balme
Mar 5, 2021·ACS Applied Materials & Interfaces·Maya MolcoAmit Sitt
Jul 16, 2021·Dalton Transactions : an International Journal of Inorganic Chemistry·Razieh MirzaeiSeyed Erfan Mirazimi

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