Highly stable nanostructured membrane electrode assembly based on Pt/Nb2 O5 nanobelts with reduced platinum loading for proton exchange membrane fuel cells

Nanoscale
Yachao ZengBaolian Yi

Abstract

Proton exchange membrane fuel cells are promising candidates for the next-generation power sources; however, poor durability and high cost impede their widespread application. To address this dilemma, a nanostructured membrane electrode assembly (MEA) based on Pt/Nb2O5 nanobelts (NBs) was constructed through hydrothermal synthesis and the physical vapour deposition method. Pt/Nb2O5 NBs were directly aligned with Nafion membrane without ionomer as a binder. The prepared catalyst layer is ultrathin and has ultralow Pt loading. A single cell performance of 5.80 kW gPt-1 (cathode) and 12.03 kW gPt-1 (anode) was achieved by the Pt/Nb2O5 NBs-based MEA (66.0 μgPt cm-2). The accelerated durability test indicates that the Pt/Nb2O5 NBs-based MEA is far more stable than conventional Pt/C-based MEA.

References

Nov 20, 2001·Nature·B C Steele, A Heinzel
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May 22, 2010·Nature Chemistry·Peter StrasserAnders Nilsson
Nov 13, 2012·Nature Materials·Dennis F van der VlietVojislav R Stamenkovic
Feb 6, 2015·Chemical Society Reviews·Yao NieZidong Wei

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