How mobile are protons in the structure of dental glass ionomer cements?

Scientific Reports
Ana R BenettiHeloisa N Bordallo

Abstract

The development of dental materials with improved properties and increased longevity can save costs and minimize discomfort for patients. Due to their good biocompatibility, glass ionomer cements are an interesting restorative option. However, these cements have limited mechanical strength to survive in the challenging oral environment. Therefore, a better understanding of the structure and hydration process of these cements can bring the necessary understanding to further developments. Neutrons and X-rays have been used to investigate the highly complex pore structure, as well as to assess the hydrogen mobility within these cements. Our findings suggest that the lower mechanical strength in glass ionomer cements results not only from the presence of pores, but also from the increased hydrogen mobility within the material. The relationship between microstructure, hydrogen mobility and strength brings insights into the material's durability, also demonstrating the need and opening the possibility for further research in these dental cements.

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Citations

Sep 3, 2016·The Review of Scientific Instruments·N TsapatsarisH N Bordallo
Mar 27, 2018·Journal of Dental Research·A K LauritsenA R Benetti
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Apr 16, 2021·Biomaterial Investigations in Dentistry·Fernanda M TsuzukiMauro L Baesso
Jun 15, 2021·Journal of the Mechanical Behavior of Biomedical Materials·Chirayu RuengrungsomJoseph E A Palamara
Mar 6, 2018·ACS Applied Materials & Interfaces·Marcella C BergHeloisa N Bordallo
Aug 31, 2021·Journal of Imaging·Nikolay KardjilovJohn Banhart

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Methods Mentioned

BETA
nuclear magnetic resonance
neutron spectroscopy
X-ray
neutron tomography

Software Mentioned

Avizo
VG Studio Max
QENS
Octopus

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