In-line and selective phase separation of medium-chain carboxylic acids using membrane electrolysis

Chemical Communications : Chem Comm
Jiajie XuLargus T Angenent

Abstract

We had extracted n-caproate from bioreactor broth. Here, we introduced in-line membrane electrolysis that utilized a pH gradient between two chambers to transfer the product into undissociated n-caproic acid without chemical addition. Due to the low maximum solubility of this acid, selective phase separation occurred, allowing simple product separation into an oily liquid containing ∼90% n-caproic and n-caprylic acid.

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Citations

Feb 26, 2016·Water Research·Leo A KucekLargus T Angenent
Feb 9, 2016·Environmental Science & Technology·Largus T AngenentHubertus V M Hamelers
Apr 2, 2016·Bioresource Technology·Shantonu RoyDeepak Pant
Apr 21, 2016·Bioresource Technology·Bastian MolitorLargus T Angenent
Oct 25, 2016·Trends in Biotechnology·Andrea SchievanoDeepak Pant
May 11, 2016·Environmental Science & Technology·Marta ComaKorneel Rabaey
Jun 25, 2016·Biotechnology for Biofuels·Byoung Seung JeonByoung-In Sang
Nov 7, 2016·Trends in Biotechnology·Pier-Luc TremblayTian Zhang
May 18, 2017·Environmental Science & Technology·Wei-Shan ChenCarolien Kroeze
Nov 3, 2017·Biotechnology for Biofuels·Tian Zhang, Pier-Luc Tremblay
Feb 18, 2016·Applied Microbiology and Biotechnology·Paul J Weimer, Richard A Kohn
Aug 3, 2017·Applied Microbiology and Biotechnology·Kun DaiRaymond J Zeng
Nov 6, 2018·Water Science and Technology : a Journal of the International Association on Water Pollution Research·Simone PerazzoliHugo M Soares
Mar 8, 2017·Frontiers in Bioengineering and Biotechnology·Stephen J AndersenKorneel Rabaey
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May 19, 2017·Frontiers in Microbiology·Edward V LaBelle, Harold D May
Jan 27, 2019·Molecules : a Journal of Synthetic Chemistry and Natural Product Chemistry·Vicky De GroofAna B Lanham
Dec 14, 2017·Angewandte Chemie·Falk Harnisch, Carolin Urban
Mar 7, 2021·Biotechnology and Bioengineering·Diana C CalvoBruce E Rittmann
Mar 30, 2021·ACS Omega·Paula Andrea HernandezBernardino Virdis
Dec 22, 2020·Environmental Science & Technology·Jiajie XuLargus T Angenent
Oct 20, 2018·Environmental Science & Technology·Catherine M SpiritoLargus T Angenent
Sep 7, 2021·Frontiers in Bioengineering and Biotechnology·Jiajie XuPascal E Saikaly

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