Lewis Acid-Base Adduct Approach for High Efficiency Perovskite Solar Cells

Accounts of Chemical Research
Jin-Wook LeeNam-Gyu Park

Abstract

Since the first report on the long-term durable 9.7% solid-state perovskite solar cell employing methylammonium lead iodide (CH3NH3PbI3), mesoporous TiO2, and 2,2',7,7'-tetrakis[N,N-di(4-methoxyphenyl)amino]-9,9'-spirobifluorene (spiro-MeOTAD) in 2012, following the seed technologies on perovskite-sensitized liquid junction solar cells in 2009 and 2011, a surge of interest has been focused on perovskite solar cells due to superb photovoltaic performance and extremely facile fabrication processes. The power conversion efficiency (PCE) of perovskite solar cells reached 21% in a very short period of time. Such an unprecedentedly high photovoltaic performance is due to the intrinsic optoelectronic property of organolead iodide perovskite material. Moreover, a high dielectric constant, sub-millimeter scale carrier diffusion length, an underlying ferroelectric property, and ion migration behavior can make organolead halide perovskites suitable for multifunctionality. Thus, besides solar cell applications, perovskite material has recently been applied to a variety fields of materials science such as photodetectors, light emitting diodes, lasing, X-ray imaging, resistive memory, and water splitting. Regardless of application areas, the...Continue Reading

References

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Sep 8, 2011·Nanoscale·Jeong-Hyeok ImNam-Gyu Park
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Citations

Feb 18, 2017·ACS Applied Materials & Interfaces·Haejun YuJyongsik Jang
Apr 20, 2017·The Journal of Physical Chemistry Letters·Jin-Wook LeeYang Yang
Jan 25, 2018·Advanced Materials·Mohammad Mahdi TavakoliZhiyong Fan
Apr 4, 2018·Advanced Materials·Xu ZhangShengzhong Frank Liu
Apr 10, 2018·Physical Chemistry Chemical Physics : PCCP·Giacomo GiorgiHiroshi Segawa
Aug 11, 2017·Chemical Society Reviews·Huan Wang, Dong Ha Kim
Feb 13, 2018·Small·Sang Il SeokNam-Gyu Park
Jun 15, 2018·Dalton Transactions : an International Journal of Inorganic Chemistry·Hong XiaoFeilong Hu
Jun 8, 2018·Angewandte Chemie·Chong GengWengang Bi
Jun 23, 2018·ChemSusChem·Yun Li, Wallace Woon-Fong Leung
Aug 31, 2018·Advanced Materials·Li Na QuanEdward H Sargent
Oct 3, 2018·Advanced Materials·Annie NgCharles Surya
Jan 4, 2019·Chemical Communications : Chem Comm·Hui-Seon KimNam-Gyu Park
Mar 28, 2019·Physical Chemistry Chemical Physics : PCCP·Ming-Chuan HsiaoFang-Chung Chen
Aug 20, 2019·Advanced Materials·Silvia G MottiAnnamaria Petrozza

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