Localized soft modes and the supercooled liquid's irreversible passage through its configuration space

The Journal of Chemical Physics
Asaph Widmer-CooperD R Reichman

Abstract

Using computer simulations, we show that the localized low frequency normal modes of a configuration in a supercooled liquid are strongly correlated with the irreversible structural reorganization of the particles within that configuration. Establishing this correlation constitutes the identification of the aspect of a configuration that determines the heterogeneity of the subsequent motion. We demonstrate that the spatial distribution of the summation over the soft local modes can persist in spite of particle reorganization that produces significant changes in individual modes. Along with spatial localization, the persistent influence of soft modes in particle relaxation results in anisotropy in the displacements of mobile particles over the time scale referred to as beta-relaxation.

References

Oct 1, 1991·Physical Review. B, Condensed Matter·H R Schober, B B Laird
Feb 4, 1991·Physical Review Letters·B B Laird, H R Schober
Oct 14, 2000·Annual Review of Physical Chemistry·M D Ediger
Oct 19, 2001·Faraday Discussions·J P DoyeS I Simdyankin
Feb 7, 2003·Physical Review Letters·R Aldrin DennyJean-Philippe Bouchaud
Aug 31, 2004·The Journal of Chemical Physics·K Vollmayr-Lee
Nov 5, 2004·Physical Review Letters·Asaph Widmer-CooperH Fynewever
Jan 25, 2005·Philosophical Transactions. Series A, Mathematical, Physical, and Engineering Sciences·David J Wales
Oct 4, 2005·Physical Review Letters·Leonardo E SilbertSidney R Nagel
Dec 31, 2005·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Katharina Vollmayr-Lee, Annette Zippelius
Feb 21, 2006·Physical Review Letters·G A AppignanesiW Kob
Apr 12, 2006·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·L A FernándezP Verrocchio
Dec 13, 2006·Physical Review Letters·Giulio BiroliDavid R Reichman
Nov 13, 2007·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Ludovic Berthier, Robert L Jack
Sep 4, 2008·Physical Review Letters·M Guerdane, H Teichler
Mar 5, 2009·Physical Review Letters·R CandelierG Biroli
May 14, 2009·Physical Review Letters·Richard S L Stein, Hans C Andersen
Jul 17, 2009·The Journal of Chemical Physics·Carolina Brito, Matthieu Wyart
Sep 17, 2008·Journal of Physics. Condensed Matter : an Institute of Physics Journal·Andreas Heuer
May 20, 2009·Journal of Physics. Condensed Matter : an Institute of Physics Journal·G A Appignanesi, J A Rodriguez Fris

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Citations

Apr 6, 2013·The Journal of Chemical Physics·Takeshi Kawasaki, Akira Onuki
Apr 6, 2013·The Journal of Chemical Physics·Glen M Hocky, David R Reichman
Dec 7, 2013·Proceedings of the National Academy of Sciences of the United States of America·Eduardo SanzPeter N Pusey
May 17, 2014·The Journal of Chemical Physics·Takeshi KawasakiAkira Onuki
Sep 18, 2014·Proceedings of the National Academy of Sciences of the United States of America·Jun DingEvan Ma
Apr 17, 2016·The Journal of Chemical Physics·S Bernini, D Leporini
Apr 4, 2015·The Journal of Chemical Physics·S BerniniD Leporini
May 26, 2016·Soft Matter·Elsen Tjhung, Takeshi Kawasaki
Dec 30, 2017·Physical Review Letters·Gang SunPeter Harrowell
Dec 12, 2012·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Hayato ShibaAkira Onuki
Jul 7, 2020·Soft Matter·Sahithya S Iyer, Anand Srivastava
Jul 23, 2020·Soft Matter·Masanari ShimadaAtsushi Ikeda
Sep 18, 2020·Soft Matter·Takeshi Kawasaki, Akira Onuki
Dec 15, 2015·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Anton Smessaert, Jörg Rottler
May 20, 2018·Physical Review. E·Rhiannon PinneyC Patrick Royall
Jun 10, 2018·The Journal of Chemical Physics·Edan Lerner, Eran Bouchbinder
Mar 12, 2016·Physical Review Letters·Smarajit KarmakarSrikanth Sastry
Dec 18, 2016·The Journal of Chemical Physics·F PuosiD Leporini
Sep 28, 2017·Physical Review. E·Pablo Montero de HijesEduardo Sanz
Apr 16, 2020·Physical Review. E·Geert KapteijnsEdan Lerner
Jun 25, 2020·Physical Review. E·Masanari ShimadaAtsushi Ikeda
Jan 20, 2017·Journal of Physics. Condensed Matter : an Institute of Physics Journal·S BerniniD Leporini
May 20, 2018·Physical Review. E·Armand BarbotSylvain Patinet
Apr 1, 2019·The Journal of Chemical Physics·Akira Onuki, Takeshi Kawasaki
May 3, 2019·The Journal of Chemical Physics·Alexander R SmithAlison B Walker
Aug 18, 2018·Physical Review Letters·Geert KapteijnsEdan Lerner
Nov 17, 2019·The Journal of Chemical Physics·Wengang ZhangFrancis W Starr
Dec 20, 2015·Reports on Progress in Physics·Smarajit KarmakarSrikanth Sastry
Aug 6, 2016·Physical Review Letters·Sylvain PatinetMichael L Falk
Dec 18, 2016·The Journal of Chemical Physics·Rhiannon PinneyC Patrick Royall
Jul 18, 2018·Physical Review. E·Fernanda P C BenettiGabriele Sicuro
May 16, 2014·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Jörg RottlerAndrea J Liu
Apr 1, 2014·Physical Review Letters·Majid MosayebiEmanuela Del Gado
May 18, 2013·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Patrick Charbonneau, Gilles Tarjus
Nov 10, 2020·Soft Matter·Masanari ShimadaAtsushi Ikeda
Sep 26, 2012·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Daniel M Sussman, Kenneth S Schweizer
Mar 1, 2021·The Journal of Chemical Physics·Hao ZhangJack F Douglas
Mar 10, 2021·The Journal of Chemical Physics·Corrado RainoneEdan Lerner
May 28, 2013·Physical Review Letters·Jader ColomboEmanuela Del Gado
Sep 13, 2014·Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics·Carl P GoodrichSidney R Nagel
Sep 28, 2010·Physical Review Letters·Ke ChenA G Yodh

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