PMID: 12786551Jun 6, 2003Paper

Molecular alignment by trains of short laser pulses

Physical Review Letters
M LeibscherH Rabitz

Abstract

We show that a dramatic field-free molecular alignment can be achieved after exciting molecules with proper trains of strong ultrashort laser pulses. Optimal two- and three-pulse excitation schemes are defined, providing an efficient and robust molecular alignment. This opens new prospects for various applications requiring macroscopic ensembles of highly aligned molecules.

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Citations

Mar 31, 2005·Annual Review of Physical Chemistry·Jiangbin Gong, Paul Brumer
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