Multidimensional Vibrational Coherence Spectroscopy

Topics in Current Chemistry
Tiago Buckup, Jérémie Léonard

Abstract

Multidimensional vibrational coherence spectroscopy has been part of laser spectroscopy since the 1990s and its role in several areas of science has continuously been increasing. In this contribution, after introducing the principals of vibrational coherence spectroscopy (VCS), we review the three most widespread experimental methods for multidimensional VCS (multi-VCS), namely femtosecond stimulated Raman spectroscopy, pump-impulsive vibrational spectroscopy, and pump-degenerate four wave-mixing. Focus is given to the generation and typical analysis of the respective signals in the time and spectral domains. Critical aspects of all multidimensional techniques are the challenges in the data interpretation due to the existence of several possible contributions to the observed signals or to optical interferences and how to overcome the corresponding difficulties by exploiting experimental parameters including higher-order nonlinear effects. We overview how multidimensional vibrational coherence spectroscopy can assist a chemist in understanding how molecular structural changes and eventually photochemical reactions take place. In order to illustrate the application of the techniques described in this chapter, two molecular system...Continue Reading

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Citations

Sep 16, 2019·The Journal of Chemical Physics·Thomas P Cheshire, Andrew M Moran
Jun 25, 2021·Journal of the American Chemical Society·Seongsoo KangDongho Kim
Feb 16, 2019·The Journal of Physical Chemistry. a·Federico J HernándezCristián G Sánchez
Dec 7, 2018·The Journal of Physical Chemistry. B·Jan Philip KraackTiago Buckup
Sep 24, 2020·The Journal of Physical Chemistry. a·Nikolaus WollscheidTiago Buckup
Sep 2, 2021·The Journal of Physical Chemistry Letters·F HainerT Buckup

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