MXene as a Charge Storage Host

Accounts of Chemical Research
Masashi OkuboAtsuo Yamada

Abstract

The development of efficient electrochemical energy storage (EES) devices is an important sustainability issue to realize green electrical grids. Charge storage mechanisms in present EES devices, such as ion (de)intercalation in lithium-ion batteries and electric double layer formation in capacitors, provide insufficient efficiency and performance for grid use. Intercalation pseudocapacitance (or redox capacitance) has emerged as an alternative chemistry for advanced EES devices. Intercalation pseudocapacitance occurs through bulk redox reactions with ultrafast ion diffusion. In particular, the metal carbide/nitride nanosheets termed MXene discovered in 2011 are a promising class of intercalation pseudocapacitor electrode materials because of their compositional versatility for materials exploration (e.g., Ti2CT x, Ti3C2T x, V2CT x, and Nb2CT x, where T is a surface termination group such as F, Cl, O, or OH), high electrical conductivity for high current charge, and a layered structure of stacked nanosheets for ultrafast ion intercalation. Various MXene electrodes have been reported to exhibit complementary battery performance, such as large specific capacity at high charge/discharge rates. However, general design strategies of...Continue Reading

References

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Citations

Jul 6, 2018·Chemical Communications : Chem Comm·Cong CuiXiaohui Wang
Nov 20, 2018·Advanced Materials·Kanit Hantanasirisakul, Yury Gogotsi
Jan 30, 2019·Chemical Record : an Official Publication of the Chemical Society of Japan ... [et Al.]·Eriko WatanabeAtsuo Yamada
Jun 25, 2019·Chemical Communications : Chem Comm·Kijae KimAtsuo Yamada
Feb 23, 2019·Nature Communications·Akira SugaharaAtsuo Yamada
Dec 10, 2019·ChemSusChem·Lu LiXitian Zhang
May 1, 2020·Chemical Communications : Chem Comm·Mark AnayeeYury Gogotsi
Jun 13, 2019·Nature Communications·Weiqian TianMahiar M Hamedi
Jul 2, 2020·Nanoscale·Geetha ValurouthuYury Gogotsi
Jul 24, 2020·Nanoscale·Muhammad Kashif Aslam, Maowen Xu
Aug 12, 2020·Chemical Society Reviews·Minmin HuZhenjiang Li
Jul 12, 2019·Chemical Science·Cyrille Costentin, Jean-Michel Savéant
Jan 19, 2021·Advanced Materials·Lingfeng GaoHans Ågren
Nov 12, 2019·Chemical Reviews·Zhongheng FuRuifeng Zhang
Jan 7, 2021·Nanomaterials·Fitri Aulia PermatasariFerry Iskandar
Apr 24, 2021·International Journal of Biological Macromolecules·Lijun YangMeifang Zhu
May 1, 2021·Nanoscale·Bingjun YangXingbin Yan
May 6, 2021·The Journal of Physical Chemistry Letters·Xining ZangRuopeng Zhang
Jun 12, 2021·Science·Armin VahidMohammadiYury Gogotsi
Aug 7, 2021·Journal of the American Chemical Society·Netanel ShpigelDoron Aurbach
Jan 16, 2020·Chemical Reviews·Tomooki HosakaShinichi Komaba
Jul 1, 2020·Chemical Reviews·Simon FleischmannVeronica Augustyn

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