New nuclear-spin-induced Cotton-Mouton effect in fluids at high DC magnetic field

Chemphyschem : a European Journal of Chemical Physics and Physical Chemistry
Guo-hua YaoFan-chen Liu

Abstract

Based on Buckingham and Pople's theory of magnetic double refraction, a theoretical expression is derived for a new Cotton-Mouton effect φ(C-M)((IB)) in liquid induced by the crossed effect between the high dc magnetic field B(0) and the nuclear magnetic moment m(z)((l)). It contains temperature-independent and -dependent parts. The latter is proportional to the product between anisotropy of polarizability and the nuclear magnetic shielding tensor. For this new effect φ(C-M)((IB)), its order in magnitude for a molecule with large polarizability anisotropy is estimated to be comparable to the nuclear-spin-induced optical Faraday rotation (NSOFR). In the multipass approach, φ(C-M)((IB)) can be eliminated by time-reversal symmetry arguments, but NSOFR is enhanced.

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Citations

Jan 21, 2014·The Journal of Chemical Physics·Li-juan Fu, Juha Vaara
Jun 8, 2013·The Journal of Chemical Physics·Li-juan Fu, Juha Vaara
Apr 10, 2014·The Journal of Chemical Physics·Juha VaaraSonia Coriani
Oct 25, 2014·Chemical Communications : Chem Comm·Michal StrakaJuha Vaara
May 28, 2014·Chemphyschem : a European Journal of Chemical Physics and Physical Chemistry·Li-Juan Fu, Juha Vaara
Apr 2, 2015·Chemphyschem : a European Journal of Chemical Physics and Physical Chemistry·Fang ChenDong-ming Chen
Aug 11, 2020·Physical Chemistry Chemical Physics : PCCP·Petr Štěpánek
May 31, 2019·Physical Chemistry Chemical Physics : PCCP·Petr Štěpánek, Sonia Coriani
Aug 28, 2019·The Journal of Physical Chemistry Letters·Petr Štěpánek, Anu M Kantola

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