Organic-Inorganic Hybrid Nanomaterials for Electrocatalytic CO2 Reduction

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Chenhuai YangWenping Hu

Abstract

Electrochemical CO2 reduction (ECR) to value-added chemicals and fuels is regarded as an effective strategy to mitigate climate change caused by CO2 from excess consumption of fossil fuels. To achieve CO2 conversion with high faradaic efficiency, low overpotential, and excellent product selectivity, rational design and synthesis of efficient electrocatalysts is of significant importance, which dominates the development of ECR field. Individual organic molecules or inorganic catalysts have encountered a bottleneck in performance improvement owing to their intrinsic shortcomings. Very recently, organic-inorganic hybrid nanomaterials as electrocatalysts have exhibited high performance and interesting reaction processes for ECR due to the integration of the advantages of both heterogeneous and homogeneous catalytic processes, attracting widespread interest. In this work, the recent advances in designing various organic-inorganic hybrid nanomaterials at the atomic and molecular level for ECR are systematically summarized. Particularly, the reaction mechanism and structure-performance relationship of organic-inorganic hybrid nanomaterials toward ECR are discussed in detail. Finally, the challenges and opportunities toward controlled ...Continue Reading

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Citations

May 26, 2021·Journal of the American Chemical Society·Bing MaGaetano Granozzi
Aug 3, 2021·Frontiers in Chemistry·Dženeta DedićWolfgang Schöfberger
Oct 9, 2021·Physical Chemistry Chemical Physics : PCCP·Chenxu ZhaoChaozheng He

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