PET-RAFT polymerisation: towards green and precision polymer manufacturing

Chemical Communications : Chem Comm
Jamie Phommalysack-LovanJiangtao Xu

Abstract

The necessity of sustainable development in the chemical industry has continuously drawn attention to find safe, environmentally friendly and atom-economic chemical processes, which is defined in the 12 principles of green chemistry. Merging photoredox catalysis and reversible addition-fragmentation chain transfer (RAFT) polymerisation, the photoinduced electron/energy transfer (PET)-RAFT process has opened up a new way of performing reversible deactivation radical polymerisation for well-defined polymer synthesis using light as an external stimulus. While providing an increased level of control (spatiotemporal, wavelength, and intensity control) over the polymerisation, PET-RAFT has many attractive attributes (abundant catalyst availability, catalyst recyclability, selectivity and oxygen tolerance) to be green and sustainable, which is intriguing for precision polymer manufacturing in industry.

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Citations

Oct 17, 2018·Macromolecular Rapid Communications·Dao LeGuillaume Delaittre
Mar 30, 2019·Chemical Communications : Chem Comm·Svante P IhrigStefan Hecht
Dec 29, 2018·Beilstein Journal of Organic Chemistry·Atsushi KagaShunsuke Chiba
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Nov 10, 2021·Macromolecular Rapid Communications·Matthias Hartlieb
Jun 16, 2021·Photochemistry and Photobiology·Matthew D ThumDaniel E Falvey

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Methods Mentioned

BETA
PISA
RAFT

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