Photocatalytic removal of gaseous nitrogen oxides using WO3/TiO2 particles under visible light irradiation: Effect of surface modification

Chemosphere
Joseph Albert MendozaJoo-Hyon Kang

Abstract

Photocatalytic nanoparticles have been receiving considerable attention for their potential use in many environmental management applications, including urban air quality control. This paper investigates the performance of surface modified WO3/TiO2 composite particles in removing gaseous nitrogen oxides (NOx) under visible light irradiation. The WO3/TiO2 composite particles were synthesized using a modified wet chemical method with different concentrations of NaOH solution used as a surface modification agent for the host TiO2 particles. The NOx removal efficiency of the WO3/TiO2 particles was evaluated using a lab-scale continuous gas flow photo-reactor with a gas contact time of 1 min. Results showed that surface modification using NaOH can enhance the photocatalytic activity of the WO3/TiO2 particles. The NOx removal efficiency of the surface modified WO3/TiO2 was greater than 90%, while that of WO3/TiO2 particles prepared by the conventional wet chemical method was ∼75%. The enhanced removal efficiency might be attributed to the formation of oxygen vacancies on the TiO2 surface, providing sites for WO3 particles to effectively bind with TiO2. However, excess amount of NaOH >3 M deteriorated the photocatalytic performance du...Continue Reading

Citations

Aug 15, 2019·Photochemical & Photobiological Sciences : Official Journal of the European Photochemistry Association and the European Society for Photobiology·Leonardo F PaulaAntonio Otavio T Patrocinio
Jan 19, 2021·Water Science and Technology : a Journal of the International Association on Water Pollution Research·Kazem NaddafiHoda Amiri

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