Progress and Perspective of Ceramic/Polymer Composite Solid Electrolytes for Lithium Batteries

Advanced Science
Song LiQuan-Hong Yang

Abstract

Solid composite electrolytes (SCEs) that combine the advantages of solid polymer electrolytes (SPEs) and inorganic ceramic electrolytes (ICEs) present acceptable ionic conductivity, high mechanical strength, and favorable interfacial contact with electrodes, which greatly improve the electrochemical performance of all-solid-state batteries compared to single SPEs and ICEs. However, there are many challenges to overcome before the practical application of SCEs, including the low ionic conductivity less than 10-3 S cm-1 at ambient temperature, poor interfacial stability, and high interfacial resistance, which greatly restrict the room temperature performance. Herein, the advances of SCEs applied in all-solid-state lithium batteries are presented, including the Li ion migration mechanism of SCEs, the strategies to enhance the ionic conductivity of SCEs by various morphologies of ICEs, and construction methods of the low resistance and stable interfaces of SCEs with both cathode and anode. Finally, some typical applications of SCEs in lithium batteries are summarized and future development directions are prospected. This work presents how it is quite significant to further enhance the ionic conductivity of SCEs by developing the no...Continue Reading

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Citations

Oct 1, 2020·Advanced Science·Tiefeng LiuJun Lu
Aug 23, 2020·Nanomaterials·Mogalahalli V ReddyKarim Zaghib
Nov 12, 2020·Angewandte Chemie·Jianxun ZhuWeidong Zhou
Mar 25, 2021·Langmuir : the ACS Journal of Surfaces and Colloids·Li TianZhiliang Liu
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Aug 12, 2021·Chemistry, an Asian Journal·Hui TangChengliang Wang
Jul 1, 2020·Chemical Reviews·Abhik BanerjeeYing Shirley Meng
Nov 21, 2020·ACS Applied Materials & Interfaces·Jianchao SunChengcheng Chen

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Methods Mentioned

BETA
ICEs
NMR

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