Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath

Physical Chemistry Chemical Physics : PCCP
Jing LiuYang Zhao

Abstract

An approach based on a non-Markovian time-convolutionless polaron master equation is used to probe the quantum dynamics of a chromophore-qubit in a super-Ohmic bath. Utilizing a measure of non-Markovianity based on dynamical fixed points, we study the effects of the environmental temperature and the coupling strength on the non-Markovian behavior of the chromophore in a super-Ohmic bath. It is found that an increase in the temperature results in a reduction in the backflow information from the environment to the chromophore, and therefore, a suppression of non-Markovianity. In the weak coupling regime, increasing the coupling strength will enhance the non-Markovianity, while the effect is reversed in the strong coupling regime.

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Citations

Nov 17, 2017·The Journal of Chemical Physics·Yaling Ke, Yi Zhao
Apr 8, 2017·The Journal of Chemical Physics·Felix VaughanFrederick R Manby
Nov 11, 2021·Physical Chemistry Chemical Physics : PCCP·An WeiLuxia Wang

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