Rational Design of Carbon-Based 2D Nanostructures for Enhanced Photocatalytic CO2 Reduction: A Dimensionality Perspective

Chemistry : a European Journal
Wee-Jun OngAbdul Rahman Mohamed

Abstract

Photocatalytic CO2 reduction is a revolutionary approach to solve imminent energy and environmental issues by replicating the ingenuity of nature. The past decade has witnessed an impetus in the rise of two-dimensional (2D) structure materials as advanced nanomaterials to boost photocatalytic activities. In particular, the use of 2D carbon-based materials is deemed as highly favorable, not only as a green material choice, but also due to their exceptional physicochemical and electrical properties. This review article presents a diverse range of alterations and compositions derived from 2D carbon-based nanomaterials, mainly graphene and graphitic carbon nitride (g-C3N4), which have remarkably ameliorated the photocatalytic CO2 performance. Herein, the rational design of the photocatalyst systems with consideration on the aspect of dimensionality and the resultant heterostructures at the interface are systematically analyzed to elucidate an insightful perspective on this pacey subject. Finally, a conclusion and outlook on the limitations and prospects of the cutting-edge research field are highlighted.

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Citations

Mar 16, 2021·Nanoscale Horizons : the Home for Rapid Reports of Exceptional Significance in Nanoscience and Nanotechnolgy·Nayeong KimJungki Ryu
May 22, 2021·Nanoscale Horizons : the Home for Rapid Reports of Exceptional Significance in Nanoscience and Nanotechnolgy·Xian Bin Lim, Wee-Jun Ong
Jun 30, 2021·Journal of Colloid and Interface Science·Jianbo WangQin Zhong

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