Recent advances in copper-catalyzed dehydrogenative functionalization via a single electron transfer (SET) process

Chemical Society Reviews
Chun ZhangNing Jiao

Abstract

Copper salts have been developed as versatile catalysts for oxidative coupling reactions in organic synthesis. During these processes, Cu-catalysts are often proposed to serve as a one-electron oxidant to promote the single-electron transfer process. Recently, the transition-metal catalyzed direct dehydrogenative transformation has attracted considerable attention. This tutorial review summarizes the recent advances in the copper-catalyzed dehydrogenative functionalization via a single electron transfer (SET) process achieving C-C, C-N, C-O, C-halogen atoms, C-P, and N-N bond formation.

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Jun 22, 2013·Chemical Reviews·Scott E AllenMarisa C Kozlowski
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