Recent Progress on Microfine Design of Metal-Organic Frameworks: Structure Regulation and Gas Sorption and Separation

Advanced Materials
Jiantang LiYunling Liu

Abstract

Metal-organic frameworks (MOFs) have emerged as an important and unique class of functional crystalline hybrid porous materials in the past two decades. Due to their modular structures and adjustable pore system, such distinctive materials have exhibited remarkable prospects in key applications pertaining to adsorption such as gas storage, gas and liquid separations, and trace impurity removal. Evidently, gaining a better understanding of the structure-property relationship offers great potential for the enhancement of a given associated MOF property either by structural adjustments via isoreticular chemistry or by the design and construction of new MOF structures via the practice of reticular chemistry. Correspondingly, the application of isoreticular chemistry paves the way for the microfine design and structure regulation of presented MOFs. Explicitly, the microfine tuning is mainly based on known MOF platforms, focusing on the modification and/or functionalization of a precise part of the MOF structure or pore system, thus providing an effective approach to produce richer pore systems with enhanced performances from a limited number of MOF platforms. Here, the latest progress in this field is highlighted by emphasizing the ...Continue Reading

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Citations

Feb 24, 2021·Dalton Transactions : an International Journal of Inorganic Chemistry·Xinyao Liu, Yunling Liu
Jul 9, 2021·ACS Applied Materials & Interfaces·Anh N HongPingyun Feng
Jun 27, 2021·Chemistry : a European Journal·Xue JiangKai-Jie Chen
Oct 6, 2021·Journal of the American Chemical Society·Weidong FanDan Zhao
Oct 20, 2021·Journal of the American Chemical Society·Zhiyong LuJoseph T Hupp

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