PMID: 18200934Jan 19, 2008Paper

Response of inorganic fine particulate matter to emission changes of sulfur dioxide and ammonia: the eastern United States as a case study

Journal of the Air & Waste Management Association
Alexandra P TsimpidiSpyros N Pandis

Abstract

A three-dimensional chemical transport model (PMCAMx) was used to investigate changes in fine particle (PM2.5) concentrations in response to changes in sulfur dioxide (SO2) and ammonia (NH3) emissions during July 2001 and January 2002 in the eastern United States. A uniform 50% reduction in SO2 emissions was predicted to produce an average decrease of PM2.5 concentrations by 26% during July but only 6% during January. A 50% reduction of NH3 emissions leads to an average 4 and 9% decrease in PM2.5 in July and January, respectively. During the summer, the highest concentration of sulfate is in South Indiana (12.8 microg x m(-3)), and the 50% reduction of SO2 emissions results in a 5.7 microg x m(-3) (44%) sulfate decrease over this area. During winter, the SO2 emissions reduction results in a 1.5 microg x m(-3) (29%) decrease of the peak sulfate levels (5.2 microg x m(-3)) over Southeast Georgia. The maximum nitrate and ammonium concentrations are predicted to be over the Midwest (1.9 (-3)g x m(-3) in Ohio and 5.3 microg x m(-3) in South Indiana, respectively) in the summer whereas in the winter these concentrations are higher over the Northeast (3 microg x m(-3) of nitrate in Connecticut and 2.7 microg x m(-3) of ammonium in New...Continue Reading

References

Nov 27, 2001·Journal of the Air & Waste Management Association·C Seigneur

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Citations

Sep 15, 2019·Environmental Science and Pollution Research International·Taciana T de A AlbuquerqueDavidson M Moreira
Jul 25, 2018·Proceedings of the National Academy of Sciences of the United States of America·Viral ShahSteven S Brown

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