Rhodium-catalyzed olefin isomerization/enantioselective intramolecular Alder-ene reaction cascade

Organic Letters
Ryuichi OkamotoKen Tanaka


The olefin isomerization/enantioselective intramolecular Alder-ene reaction cascade was achieved by using a cationic rhodium(I)/(R)-BINAP complex as a catalyst. A variety of substituted dihydrobenzofurans and dihydronaphthofurans were obtained from phenol- or naphthol-linked 1,7-enynes, respectively, with good yields and ee values.


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