Simultaneous Stress and Field Control of Sustainable Switching of Ferroelectric Phases

Scientific Reports
P FinkelS E Lofland

Abstract

In ferroelectrics, manifestation of a strong electromechanical coupling is attributed to both engineered domain morphology and phase transformations. However, realization of large sustainable and reversible strains and polarization rotation has been limited by fatigue, nonlinearity and hysteresis losses. Here, we demonstrate that large strain and polarization rotation can be generated for over 40 × 10(6) cycles with little fatigue by realization of a reversible ferroelectric-ferroelectric phase transition in [011] cut Pb(In1/2Nb1/2)O3-Pb(Mg1/3Nb2/3)O3-PbTiO3 (PIN-PMN-PT) relaxor ferroelectric single crystal. Direct tuning of this effect through combination of stress and applied electric field, confirmed both macroscopically and microscopically with x-ray and Raman scattering, reveals the local symmetry while sweeping through the transition with a low applied electric field (<0.2 MV/m) under mechanical stress. The observed change in local symmetry as determined by x-ray scattering confirms a proposed polarization rotation mechanism corresponding to a transition between rhombohedral and orthorhombic phases. These results shed more light onto the nature of this reversible transformation between two ferroelectric phases and advance...Continue Reading

References

Aug 1, 1986·Physical Review. B, Condensed Matter·A AminL E Cross
Sep 16, 2000·Physical Review Letters·R GuoG Shirane
Jun 19, 2007·IEEE Transactions on Ultrasonics, Ferroelectrics, and Frequency Control·Ahmed AminLynn Ewart
Sep 28, 2010·Physical Review Letters·Sen YangJianrong Gao

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Citations

Oct 6, 2018·Nature Communications·Huilong HouIchiro Takeuchi

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Methods Mentioned

BETA
x-ray diffraction
X-ray

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