Smart, Piezo-Responsive Polyvinylidenefluoride/Polymethylmethacrylate Surface with Triggerable Water/Oil Wettability and Adhesion

ACS Applied Materials & Interfaces
Olga GuselnikovaOleksiy Lyutakov

Abstract

The design of smart surfaces with externally triggerable water/oil wettability and adhesion represents one of the most up-to-date challenges in the field of material science. In this work, the intelligent surface with electrically triggerable wettability and water/oil adhesion is presented. As a basic material background exhibiting electric field (EF) sensitivity, the piezo-responsive polymethylmethacrylate/polyvinylidenefluoride polymer fibers were used. To expand the available range of water/oil contact angles (CAs) and adhesion, the fibers were grafted with hydrophilic or hydrophobic functional groups using diazonium chemistry. The fiber functionality was evaluated using the static CA and wettability hysteresis measurements (increasing/decreasing drop volume and tilting angles), drops adhesion/repellence and graphite self-cleaning test performed with and without the application of EF. It was found that the proposed method enables tuning the surface wettability in the superhydrophobic/superoleophobic-hydrophilic/oleophilic range and changing of surface properties from low adhesive to high adhesive for water and oil. More convincing results were achieved in the case of fiber surface modification by ADT-C8F17, which may result ...Continue Reading

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Citations

Oct 2, 2019·Advanced Materials·Christoph ButenBart Jan Ravoo
Jul 25, 2019·Scientific Reports·Peter ThurgoodKhashayar Khoshmanesh
May 1, 2021·Polymers·Li JingchengRituparna Ghosh
Jun 26, 2021·Journal of the American Chemical Society·Shuaijun PanFrank Caruso
Jun 17, 2021·Journal of Bionic Engineering·Shuyi LiLuquan Ren
May 20, 2020·ACS Applied Materials & Interfaces·Jingyu WangXudong Wang
Jan 1, 2021·ACS Applied Materials & Interfaces·Weiwei ZhengYuekun Lai

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