Solar-Driven Production of Hydrogen Peroxide from Water and Dioxygen

Chemistry : a European Journal
Shunichi FukuzumiWonwoo Nam

Abstract

Hydrogen peroxide, which is a green oxidant and fuel, is produced by a two-electron/two-proton reduction of dioxygen, two-electron/two-proton oxidation of water, or a combination of four-electron/four-proton or/and two-electron/two-proton oxidation of water and two-electron/two-proton reduction of dioxygen. There are many reports on electrocatalysts for selective two-electron/two-proton reduction of dioxygen to produce hydrogen peroxide instead of four-electron/four-proton reduction of dioxygen to produce water. As compared with the two-electron/two-proton reduction of dioxygen to produce hydrogen peroxide, fewer catalysts are known for the selective two-electron/two-proton oxidation of water to produce hydrogen peroxide instead of four-electron/four-proton oxidation of water to evolve dioxygen. Thus, solar-driven production of hydrogen peroxide mainly consists of the catalytic four-electron/four-proton oxidation of water and the catalytic two-electron/two-proton reduction of dioxygen. The overall reaction is the solar-driven oxidation of water by dioxygen to produce hydrogen peroxide. Either or both the four-electron/four-proton or/and the two-electron/two-proton oxidation of water and the two-electron/two-proton reduction of ...Continue Reading

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Citations

Dec 19, 2018·Dalton Transactions : an International Journal of Inorganic Chemistry·Shunichi FukuzumiWonwoo Nam
Mar 22, 2019·Chemical Society Reviews·Biaobiao Zhang, Licheng Sun
Nov 16, 2019·Physical Chemistry Chemical Physics : PCCP·Artem PimachevYuri Dahnovsky
Jan 17, 2020·Chemical Communications : Chem Comm·Maciej Gryszel, Eric Daniel Głowacki
Oct 2, 2019·Angewandte Chemie·Huilin HouXiwang Zhang
Jun 23, 2020·Physical Chemistry Chemical Physics : PCCP·Artem PimachevYuri Dahnovsky
Apr 25, 2020·Chemistry : a European Journal·Takahiko KojimaTomoya Ishizuka
Feb 16, 2020·Nature Communications·Bastien BissaroVincent G H Eijsink
Apr 29, 2021·Chemphyschem : a European Journal of Chemical Physics and Physical Chemistry·Justyna KaliszMarcin Opallo
Jul 23, 2021·Journal of the American Chemical Society·Yasuhiro ShiraishiTakayuki Hirai

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