Strong piezoelectricity in (1 - x)(K0.4Na0.6)(Nb0.96Sb0.04)O3-xBi0.5K0.5Zr1-ySnyO3 lead-free binary system: identification and role of multiphase coexistence

ACS Applied Materials & Interfaces
Ting ZhengXiaojie Lou

Abstract

Here we report a strong piezoelectric activity in (1 - x)(K0.4Na0.6)(Nb0.96Sb0.04)O3-xBi0.5K0.5Zr1-ySnyO3 lead-free ceramics by designing different phase boundaries. The phase boundaries concerning rhombohedral-orthorhombic-tetragonal (R-O-T) and rhombohedral-tetragonal (R-T) multiphase coexistence were attained by changing BKZS and Sn contents and then were identified by the X-ray diffraction patterns as well as temperature-dependent permittivity and ν1 Raman modes associated with BO6 perovskite octahedron. A high strain (strain = 0.21-0.28% and d33* = 707-880 pm/V) and a strong piezoelectric coefficient (d33 = 415-460 pC/N) were shown in the ceramics located at the multiphase coexistence region. The reported results of this work are superior to that (d33* ∼ 570 pm/V and d33 ∼ 416 pC/N) of the textured (K,Na,Li)(Nb,Ta,Sb)O3 ceramics [Nature 2004, 432, 84]. We believe that the material system of this work will become one of the most promising candidates for piezoelectric actuators.

References

Mar 1, 1971·Archives of Otolaryngology·B F Jaffe
Nov 2, 2004·Nature·Yasuyoshi SaitoMasaya Nakamura
Jan 22, 2014·Nature Communications·Tom T A LummenVenkatraman Gopalan
Feb 7, 2014·Journal of the American Chemical Society·Xiaopeng WangXiangjian Wang
May 23, 2014·Dalton Transactions : an International Journal of Inorganic Chemistry·Ting ZhengXiaojie Lou
Jun 25, 2014·Dalton Transactions : an International Journal of Inorganic Chemistry·Ting ZhengXiangjian Wang

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Citations

Aug 25, 2015·ACS Applied Materials & Interfaces·Ting ZhengXiaojie Lou
Jan 9, 2020·Chemical Society Reviews·Xiang LvJiagang Wu
Jan 2, 2016·Materials·María Elena Villafuerte-CastrejónLorena Pardo

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