Surface-confined single-layer covalent organic frameworks: design, synthesis and application

Chemical Society Reviews
Daling CuiFederico Rosei

Abstract

Two-dimensional (2D) nanomaterials, such as graphene and single layer covalent organic frameworks (sCOFs) are being widely studied due to their unusual structure/property relationships. sCOFs typically feature atomic thickness, intrinsic nanoscale porosity and a crystalline lattice. Compared to other organic 2D materials, sCOFs exhibit major advantages including topological designation and constitutional tunability. This review describes the state of the art of surface-confined sCOFs, emphasizing reticular design, synthesis approaches, and key challenges related to improving quality and exploring applications.

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Citations

Jan 21, 2021·ACS Applied Materials & Interfaces·Indulekha MukkattAyyappanpillai Ajayaghosh
Jul 9, 2021·Dalton Transactions : an International Journal of Inorganic Chemistry·Markus Lackinger
Dec 8, 2020·Journal of the American Chemical Society·Halleh B BalchFeng Wang
Nov 9, 2021·The Journal of Physical Chemistry Letters·Zhenzhe ZhangRustam Z Khaliullin

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Methods Mentioned

BETA
delamination
scanning
X-ray
thermal treatment
scanning electron microscopy
differential scanning calorimetry

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