Synthesis and Post-Synthesis Transformation of Germanosilicate Zeolites

Angewandte Chemie
Maksym OpanasenkoJiří Čejka

Abstract

Zeolites are one of the most important heterogeneous catalysts, with a high number of large-scale industrial applications. While the synthesis of new zeolites remain rather limited, introduction of germanium has substantially increased our ability to not only direct the synthesis of zeolites but also to convert them into new materials post-synthetically. The smaller Ge-O-Ge angles (vs. Si-O-Si) and lability of the Ge-O bonds in aqueous solutions account for this behaviour. This Minireview discusses critical aspects of germanosilicate synthesis and their post-synthesis transformations to porous materials.

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Citations

Oct 10, 2020·Chemical Science·Daniel N RainerRussell E Morris
Jun 22, 2021·Dalton Transactions : an International Journal of Inorganic Chemistry·Daniel N Rainer, Russell E Morris
Jul 6, 2021·Materials Advances·Ondřej VeselýJiří Čejka
Dec 17, 2021·Journal of the American Chemical Society·Rishabh JainJeffrey D Rimer

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